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Quasi-elastic neutron scattering study of hydrated DNA.
Beta, I. A.; Michalarias, I.; Ford, R. C.; Li, J. C.; Bellissent-Funel, M.-C
Chemical Physics. 2003;292:451-454.
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Abstract
Dynamics of water around DNA mols. was studied by incoherent quasi-elastic neutron scattering. The mean residence time is about 10 times higher than for liq. water indicating that mobility of water adsorbed on DNA is reduced very significantly. The mean residence time increases from 10 ps for the sample with 2.5 g water/g DNA to 18 ps for a water content of 0.31 g water/g DNA. The activation energy of diffusion for water in hydrated DNA samples detd. by the Arrhenius plot is Ea=6.9 kcal/mol, a value significantly higher than 4.2 kcal/mol estd. for liq. water. [on SciFinder (R)]
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